Scientific Requirements Demand a New Generation of Light Source
In order to have a major impact on the fundamental questions, scientific goals and research objectives of the future, a new generation of light source is required. The necessary capabilities of such a source is substantially beyond those of both third-generation storage rings and the x-ray FELs that are now planned or under construction. The two most challenging performance requirements that must be met simultaneously are: ultrafast temporal resolution (driven by the fundamental time scales of correlation phenomena in matter), and high average flux (driven by the required measurement precision/resolution). Table 1 specifies the various performance requirements and summarizes the research areas that are the primary drivers of each requirement.
Table 1
Table 1 Performance requirements and research needs driving specifications for future light sources
Performance Category |
Quantification |
Required for: |
Ultrafast
Time Resolution |
<100
fs |
All dynamics studies - attosecond to picosecond time scales - duration/bandwidth control |
High Repetition Rate |
10-100 KHz |
Time-resolved spectroscopy - high repetition rate for signal averaging - repetition rate limited by sample recovery/replacement - flux per pulse limited by damage and non-linear efffects Inelastic x-ray scattering Lensless imaging |
High Average Flux |
~1015 ph/s/0.1%
BW |
Time-resolved spectroscopy X-ray emission spectroscopy—RIXS/XES (at 0.5 eV resolution) - flux per pulse limited by damage and nonlinear effects |
Very High Average Flux |
>>1015 ph/s/0.1%
BW |
Inelastic x-ray scattering—IXS X-ray emission spectroscopy—RIXS/XES (<10 meV resolution) Lensless imaging - flux per pulse limited by damage and nonlinear effects |
Tunability |
100 eV – 10 KeV |
X-ray spectroscopy (electronic/atomic structure) - soft x-ray: XANES, EXAFS (TM L-edges) - hard x-ray: EXAFS (TM K-edges) |
Polarization Control |
adjustable circular/linear |
All x-ray dichroism spectroscopy |
Coherence |
Full transverse and longitudinal |
Energy resolution (temporal transform limit) Chirped/shaped pulse experiments Lensless imaging (transverse coherence) |
Stability |
<10% pulse amplitude <0.1sx,y alignment |
Extraction of small signals from background |